Short answer: No.
Long answer: if you were planning on forming the furazan, you might be able to oxidize the two methyl groups to carboxyl groups, and then
decarboxylate the compound during nitration.
Catalytic vapor phase oxidation of acetone to acetaldehyde is possible (with copper foil),
http://lecturedemos.chem.umass.edu/chemReactions5_4.html
so I would think the same might be possible with diacetyl (butane-2,3-dione) to get glyoxal, though I suspect the yields might not be very good.
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