"We report that Alpha-H2CO3 can be sublimated and recondensed without decomposition into CO2 and H2O... To examine the stability of H2CO3, we prepared
a film of crystalline H2CO3 on a CsI window by sequentially depositing layers of glassy methanolic solutions of 0.1 M KHCO3 and of is similar to 2 M
HCl in the form of droplets, then by heating in vacuo from 78 to 200 K to induce protonation of HCO3, sup - and removal of solvent and excess HCl. The
infrared spectrum of the film recorded at 200 K is characteristic for Alpha-H2CO3 (Fig. 1, curves 1) ( 10-12). The high crystallinity of the film is
indicated by sharpening of bands and pronounced bandsplitting ( 12). The HCO3, sup - was completely protonated, as indicated by the absence of the
intense HCO3, sup - band centered at is similar to 1647 cm-1 ( 10, 12). The CsI window with the H2CO3 film was removed from the apparatus together
with its holder by breaking the vacuum with Ar (99.999%), and it was then stored in liquid N2." |